Can I upload file that it's size over 100 GigaBytes?
This is not possible: 100GB is the max amount of data you can upload/generate in a single instance/Job.
If it's possible, you can split your dataset into 2 shards and upload it as 2 different datasets, or different version of the same dataset. Then you can train in 2 times. I'm sorry for the bad experience, we will improve this in the next weeks/months.